Two-photon spectra of quantum emitters. A. González-Tudela, F. P. Laussy, C. Tejedor, M. J Hartmann and E. del Valle in New J. Phys. 15:033036 (2013).
This paper introduces for the first time—and computes explicitely for various cases—the two-photon correlation spectrum (or "two-photon spectrum" as per the nomenclature of the paper), that is, the 2D landcape of photon correlations when retaining their frequency degree of freedom.
We made a "video abstract" to explain the main idea:
This is, for instance, the 2PS (two-photon spectrum) for the Mollow triplet:
We understood the triplet of red antidiagonal lines right away (they are leapfrog processes) but it would take another decade for us to figure out the blue circles![1]
The two-photon spectrum has been measured experimentally for the first time by Peiris et al.,[2] which is the most interesting case, and shortly after that by Silva et al.[3] but for something with much less quantum structure.
Such 2D structures remain ignored by the bulk of quantum opticians, who fail to understand that to look at two-photon observables, one must look at two-photon spectra. In this way, peopled remained oblivious to the strongly-correlated emission away from the spectral peaks that, if you Purcell-enhance it, gives rise to a new regime of quantum emission.[4]